Download PDF by John von Neumann: Collected works. Vol.3 Ring of operators

By John von Neumann

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18) (K = Ka for nearly prolate, K = Kc for nearly oblate). 2 Magnetic-interaction constants, defining equations The spectroscopic determination of the spin-rotation-, spin-spin-, and nuclear-shielding parameters of diamagnetic molecules compiled here requires a resolving power of the order of l…10 kHz. This can be achieved with the MWFT method or with molecular-beam techniques in current use so that the reader will find several molecules in the tables below where some of the pertinent parameters have been determined.

Ref. p. 21 Note that authors sometimes use the notation Mk instead of Ck for the spin-rotation tensor. It is appropriate to refer these quantities to the molecular principal-axis system (a, b, c). In this way, the tensor k kl k components Cgg c , Dgg c , g gg c , [ gg c and V gg c become uniquely defined molecular properties (g, gƍ = a, b, c). However, only the diagonal tensor components are useful in analyzing hfs spectra as non-diagonal terms, g z gƍ do not enter matrix elements diagonal in J, and higher-than-first-order rotational perturbations of H are barely observable.

Pol. A 104 (2003) 415. : J. Chem. Phys. 119 (2003) 7749. 1007/978-3-642-10400-8_3 © Spr inger 2011 32 256 C3HHeN 2-Propynenitrile - helium (1/1) 256 C3HHeN 2-Propynenitrile - helium (1/1) Constants: (A, B, C), χgg(14N, D) For definitions, see Introduction H C C C N He Structural parameters: See [05Top] (T-shaped complex). : J. Chem. Phys. 123 (2005) 064303. : 4452-08-8 C N C O Structural parameters: See [04Hah]. 381(17) Other centrifugal distortion constants fixed to the values of the parent isotopologue.

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Collected works. Vol.3 Ring of operators by John von Neumann


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